This number seems definitely spoofed. I've never seen a 240 exchange within a 301 area code. The call came to my cell and I didn't answer and no message was left on 10/4/14 at 2:07PM.
There is a 301 240 exchange, but the 4100 block of extensions is currently unassigned. This as a spoofed ANI. This block is unassigned in the NANPA database.